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Experimental study on the in-plane thermal conductivity of Au nanofilms

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【作者】 TAKAHASHI KojiIKUTA TatsuyaFUJII Motoo

【Author】 CAO Bingyang, ZHANG Qingguang, ZHANG Xing, TAKAHASHI Koji, IKUTA Tatsuya, QIAO Wenming and FUJI I Motoo ( Key Laboratory for Thermal Science and Power Engineering of Ministry of Education, Department of Engineering Mechanics, Ts-inghua University, Beijing 100084, China; Graduate School of Engineering, Kyushu University, Fukuoka 812-8581, Japan; Institute for Materials Chemistry and Engineering, Kyushu University, Kasuga 816-8580, Japan)

【机构】 Graduate School of Engineering Kyushu UniversityFukuoka 812-8581JapanGraduate School of EngineeringKyushu UniversityInstitute for Materials Chemistry and EngineeringKasuga 816-8580

【摘要】 <正>The in-plane thermal conductivity of Au nanofilms with thickness of 23 nm, which are fabricated by the electron beam-physical vapor deposition method and a suspension technology, is experimentally measured at 80-300 K by a one-dimensional steady-state electrical heating method. Strong size effects are found on the measured nanofilm thermal conductivity. The Au nanofilm in-plane thermal conductivity is much less than that of the bulk material. With the increasing temperature, the nanofilm thermal conductivity increases. This is opposite to the temperature dependence of the bulk property. The Lorenz number of the Au nanofilms is about three times larger than the bulk value and decreases with the increasing temperature, which indicates the invalidity of the Wiedemann-Franz law for metallic nanofilms.

【Abstract】 The in-plane thermal conductivity of Au nanofilms with thickness of 23 nm, which are fabricated by the electron beam-physical vapor deposition method and a suspension technology, is experimentally measured at 80-300 K by a one-dimensional steady-state electrical heating method. Strong size effects are found on the measured nanofilm thermal conductivity. The Au nanofilm in-plane thermal conductivity is much less than that of the bulk material. With the increasing temperature, the nanofilm thermal conductivity increases. This is opposite to the temperature dependence of the bulk property. The Lorenz number of the Au nanofilms is about three times larger than the bulk value and decreases with the increasing temperature, which indicates the invalidity of the Wiedemann-Franz law for metallic nanofilms.

【基金】 Supported by National Natural Science Foundation of China (Grant No. 50606018)
  • 【文献出处】 Progress in Natural Science ,自然科学进展(英文版) , 编辑部邮箱 ,2007年02期
  • 【分类号】O484.4
  • 【下载频次】53
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