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Ti掺杂对La1.2Ca1.8Mn2-xTixO7磁电阻的影响

Ti DOPING EFFECTS ON MAGNETORESISTANCE IN THE LAYERED PEROVSKITE La1.2 Ca1.8 Mn2-x TixO7

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【作者】 陈勤潘亚林

【Author】 Chen Qin (Department of Materials Science and Engineering,University of Science and Technology of China,Hefei 230026) Pan Yalin (Deparment of Environmental Engineering and Electron,Anhui Institute of Architecture,Hefei,230022)

【机构】 中国科学技术大学材料科学与工程系!合肥230026安徽建筑工业学院环境工程与电子系!合肥230022

【摘要】 研究层状钙钛矿结构锰氧化物 La1 .2 Ca1 .8Mn2 - x Tix O7( x=0 .0 0 ,0 .0 5,0 .1 0 )块状样品磁电阻性质 ,发现 Mn位掺杂 Ti4+ 离子使材料电阻率上升 ,电阻率峰值温度 Tp 降低 ,Tp 附近及低温下磁阻增加 ;当 x=0 .1 0时 ,材料在所测温区表现为类绝缘态 ,但在 H=0 .5T外场下可观察到场致的金属 -绝缘体转变 ,同时获得磁电阻 ( MR=〔ρ( H) -ρ( 0 )〕/ρ( 0 ) )高达 -4 3 %。对以上结果的解释应是同时考虑在层状钙钛矿材料内的各向异性交换作用和因磁结构被破坏而产生的具有不同磁相关长度的区域的共存

【Abstract】 The properties of magnetoresistance of the layered perovskite manganite La 1.2 Ca 1.8 Mn 2-x Ti xO 7(x=0.00,0.05,0.10)have been studied.The doping of Ti 4+ ion at manganese site exhibits an increase in resistivity,a decrease in the resistivity peak temperature and an enhancement of the magnetoresistance low temperature in the compounds.When x=0.10,the system behaves insulator-like over the whole measuring temperature range,but a metal-insulator transition induced by a external field of 0.5T was observed,which causes a large magnetoresistance (MR=〔ρ(H)-ρ(0)〕/ρ(0))of-43%.The above results can be explained in terms of the anisotropic exchange interaction in layered perovskites and the coexistence of the regions with different magnetic coherence length originating from the disorder of magnetic structure.

  • 【文献出处】 安徽建筑工业学院学报(自然科学版) ,JOURNAL OF ANHUI INSTITUTE OF ARCHITECTURE , 编辑部邮箱 ,2000年02期
  • 【分类号】TM271
  • 【被引频次】1
  • 【下载频次】22
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