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Zn掺杂La2CuO4热电势和磁化率研究

Study on the thermopower and magnetic properties of Zn doped La2CuO4

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【作者】 杨宏顺李鹏程柴一晟余旻李志权李明德曹烈兆闻海虎龙云泽陈兆甲

【Author】 JZ]Yang Hong Shun 1) Li Peng Cheng 1) Chai Yi Sheng 1) Yu Min 1) \ Li Zhi Quan 1) Li Ming De 1) Cao Lie Zhao 1) \ Wen Hai Hu 2) Long Yun Ze 2) Chen Zhao Jia 2) 1) (Structural Resear

【机构】 中国科学技术大学结构分析开放实验室中国科学院

【摘要】 测量了La2 CuO4 掺Zn样品在不同降温速率下 (330K保温 0 5h ,然后分别以 6K h ,0 2K s的速度降到 8K)的直流磁化率和热电势 .实验结果表明 ,反铁磁温度TN 不随降温速率变化而变化 ,其直流磁化率也未受很大影响 .高温热电势弱的温度依赖关系表明为极化子气体的贡献 .热电势在转折温度Tdrop之下的快速降低是由于二维反铁磁涨落的贡献 .热电势在更低温度的拐点TS 与载流子的局域化有关 .降温速率变化时 ,Tdrop和TS 都有明显的变化 .Zn掺杂对Tdrop和TS 没有明显影响 ,但导致了更强的载流子局域化 .讨论了上述现象产生的物理图像

【Abstract】 We report on a study of the temperature dependence of thermoelectric power and DC susceptibility of Zn doped La 2CuO 4 throngh slow cooling and slow warming after quenching (6K/h,and 0.2K/s respectively).The antiferromagnetic (AF) transition temperature T N does not change with changing cooling rates and the dc susceptibility for La 2CuO 4 is not much affected.The high temperature thermopower is weakly temperature dependent,suggesting the hopping contribution of polarons.The rather rapid linear decrease in the thermopower below T drop is attributed to the contribution of the two dimensional AF fluctuations.The spinodal in thermopower at lower temperature is confirmed to be related with the localization of the charge carriers.The T drop and T S are obviously changed by changing cooling rates while they are not affected much by Zn doping.However,the Zn doping results in a stronger localization of charge carriers.In this paper,we discuss the physical origins related to above phenomena.

【关键词】 La2CuO4直流磁化率热电势
【Key words】 La 2CuO 4thermopowermagnetic susceptibility
【基金】 国家重点基础研究专项基金 (批准号 :19990 64 6)资助的课题~~
  • 【文献出处】 物理学报 ,Acta Physica Sinica , 编辑部邮箱 ,2002年09期
  • 【分类号】O511.4
  • 【下载频次】105
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