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氦同位素4 K低温吸附分离特性研究

Research on cryogenic adsorptive separation characteristics of helium isotopes at 4 K

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【作者】 储逸群李殷飞陈欢屈千喜徐伟鹏徐冬贾朋李来风

【Author】 Chu Yiqun;Li Yinfei;Chen Huan;Qu Qianxi;Xu Weipeng;Xu Dong;Jia Peng;Li Laifeng;Key Laboratory of Cryogenic Science and Technology, Technical Institute of Physics and Chemistry,Chinese Academy of Sciences;University of Chinese Academy of Sciences;

【通讯作者】 贾朋;

【机构】 中国科学院理化技术研究所低温科学与技术全国重点实验室中国科学院大学

【摘要】 为发展自主可控的3He/4He分离技术,研制了一套以GM制冷机为冷源的氦同位素低温吸附分离实验平台,主要部件包括低温控制单元、气体控制单元以及吸附柱单元。选用椰壳活性炭作为吸附剂,通过动态吸附-解吸循环实验探究其对3He/4He混合气体的分离特性。实验结果表明:在4.2 K的吸附温度下,3He在椰壳活性炭上的动态吸附性能显著优于4He;经过3次连续的吸附-解吸循环后,所得解吸气体中3He的丰度由初始值提升至99.93%。

【Abstract】 To advance the development of autonomous and controllable 3He /4He separation technology, an experimental cryogenic adsorption separation platform for helium isotopes was established, utilizing a GM cryocooler as the cold source. The primary components of the system include a cryogenic control unit, a gas control unit, and an adsorption column unit. Coconut shell activated carbon was selected as the adsorbent, and its separation characteristics for 3He /4He gas mixtures were investigated through dynamic adsorption-desorption cycle experiments. The experimental results indicate that at an adsorption temperature of 4. 2 K, the dynamic adsorption performance of 3He on coconut shell activated carbon is significantly superior to that of 4He. After three consecutive adsorption-desorption cycles, the 3He abundance in the desorbed gas increased from the initial value to 99. 93%.

【基金】 中国科学院中央级科研院所科学研究条件专项基金(GSZXKYZB2025023)
  • 【分类号】TL921;O647.3;TB651
  • 【下载频次】17
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