【摘要】 固态锂金属电池进行充放电时，表面粗糙的锂电极和固态电解质界面上产生的应力对锂枝晶的产生有重要影响．本文通过建立电极与电解质组成的弹性体的力学模型，具体针对二维三角函数波形的粗糙界面，对于各向同性线弹性材料，研究了电极与电解质界面的应力．基于二维傅里叶变换，获得了变换域中界面处的应力和位移之间的关系，通过逆变换并结合边界条件和界面连续性条件，最终得到了二维情况下电极和电解质界面应力的解析解．当界面沿一个方向的表面粗糙度波数为零时，该界面应力解可以退化为已有的一维情况的解．通过算例分析了电解质和电极材料参数对界面应力大小的影响．更多还原

【Abstract】 During the charge and discharge processes of solid-state lithium metal batteries, the stress generated at the interface between the rough surfaces of the lithium electrode and solid-state electrolyte plays a crucial role in the formation of lithium dendrites. In this paper, a mechanical model is established by considering the electrode and electrolyte as elastic bodies.Specifically, the stress at the interface of a two-dimensional sinusoidal rough interface is investigated for isotropic linear elastic materials. Using a two-dimensional Fourier transform, the relationship between stress and displacement at the interface in the transform domain is obtained. By applying the inverse transform and incorporating boundary conditions and interface continuity conditions, an analytical solution for the interfacial stress in two dimensional conditions is derived. When the wavenumber of surface roughness in one direction of the interface is zero, the two-dimensional interfacial stress solution degrades to the onedimensional case. Subsequently, the analytical solution is used to analyze the influences of the material parameters of the electrolyte and electrode on the magnitude of the interfacial stress.更多还原