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保定市PM2.5和臭氧复合污染特征及输送路径分析

Analysis of Characteristics and Transport Pathways of PM2.5 and Ozone Composite Pollution in Baoding City

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【作者】 宋晓伟; 孔媛; 郝永佩; 朱晓东; 王京伟; 程鹏;

【Author】 SONG Xiaowei;KONG Yuan;HAO Yongpei;ZHU Xiaodong;WANG Jingwei;CHENG Peng;College of Resources and Environment, Shanxi University of Finance & Economics;State Key Laboratory of Pollution Control and Resource Reuse, School of the Environment, Nanjing University;

【机构】 山西财经大学资源环境学院; 南京大学环境学院,污染控制与资源化研究国家重点实验室;

【摘要】 为探究京津冀地区大气污染典型城市保定市PM2.5和臭氧复合污染现状,文章基于2015-2022年大气污染物浓度及气象参数进行统计分析,探究了保定市PM2.5和O3不同时段的浓度变化特征,并运用后向轨迹模型、潜在源贡献因子法和浓度权重轨迹法探究气团传输对PM2.5和O3污染的贡献。结果表明:保定市2015-2022年PM2.5浓度逐年下降,而O3浓度呈波动上升趋势;季节上PM2.5浓度表现为冬季高、夏季低的特征,O3浓度则表现出相反特征。研究期间PM2.5-O3复合污染日和PM2.5单污染日的天数均呈下降趋势,且天数集中出现在4-9月和10月-次年3月,而O3单污染日天数则呈上升趋势;PM2.5-O3复合污染极易出现于温度为20.8~26.7℃、相对湿度为59.0%~77.5%、风速较低的气象条件下。保定市复合污染期间受来自西北方向长距离及偏南方向短距离气流影响显著;复合污染和PM2.5单污染期间的PM2.5潜在源区主要集中在保定市周边以及贯穿覆盖内蒙古自治区西部到安徽北部的西北-东南方向的污染区域带上,复合污染状况下O3和O3单污染期间主要受到城市周边区域、河南中北部、山东中西部及安徽北部影响。

【Abstract】 In order to explore the composite pollution status of PM2.5 and ozone in Baoding City,a typical air polluted city in the Beijing-Tianjin-Hebei region,this study analyzes the variation characteristics at different periods,concentration relation?ships and influencing factors of PM2.5 and O3 in Baoding,while investigating the contribution of air mass transport to PM2.5 and O3 pollution using trajectory cluster analysis,the potential source contribution function and concentration-weighted trajectory method,based on PM2.5 and O3 concentrations as well as meteorological parameters and Global Data Assimilation System data collected from 2015 to 2022.The results show that from 2015 to 2022,the PM2.5 concentration decreased year by year,with a higher concentration in winter than in summer;the O3 concentration showed a fluctuating upward trend,with a higher concen?tration in summer than in winter.Both PM2.5-O3 composite pollution days and PM2.5 single pollution days showed a downward trend,with high concentration appearing in April-September and October-March of the following year.PM2.5-O3 compos?ite pollution was very likely to occur under the following meteorological conditions:a temperature of 20.8~26.7℃,a humidity of 59.0%~77.5%,and low wind speed.The cluster analysis showed that during the period of composite pollution,Baoding would be significantly affected by the long-distance airflow from the northwest and the short-distance airflow from the south.The PSCF and CWT analysis showed that the potential source areas were mainly concentrated around Baoding and in the northwest-southeast polluted regions,ranging from western Inner Mongolia to northern Anhui,in PM2.5 composite pollu?tion conditions and during PM2.5single pollution periods.On the other hand,the pollution was mainly concentrated around the urban surrounding regions,central and northern Henan,central and western Shandong and northern Anhui in O3 composite pol?lution conditions and during O3 single pollution periods.

【基金】 国家自然科学基金项目(72104132);教育部人文社会科学基金项目(21YJCZH136);2024年山财学者学术拔尖骨干人才科研项目(BY-Z01059)
  • 【文献出处】 环境科学与技术 ,Environmental Science & Technology , 编辑部邮箱 ,2025年05期
  • 【分类号】X51
  • 【下载频次】73
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