Determination of the half-life of ^184gRe and the isomeric ratio of ^184m,gRe induced by D-T neutrons

【摘要】 The isomeric ratio of ^184m,gRe and the half-life of ^184gRe were measured in the ¹⁸⁵Re（n,2n） ¹⁸⁴Re reaction at 14.8 MeV,and the uncertainty was discussed in detail.The measurements were performed using the activation method implemented for a rhenium sample using the K-400 neutron generator at the Chinese Academy of Engineering Physics（CAEP）.Isomeric state and ground state nuclei of ¹⁸⁴Re were identified by their γ-ray spectra.To eliminate the effect of the γ-ray emitted from the isomer on the counting of the ground state characteristic peaks,the isomeric ratio of ^184m,gRe was calculated to be 0.29±0.11 according to the neutron activation cross-section formula.This result is consistent with previous data within the uncertainty and can be used to determine parameters that characterize the dependence of the level density on the excitation energy and angular momentum.Through exponential function fitting and a detailed discussion of the uncertainty evaluation,the half-life of ^184gRe was determined as 35.43 ± 0.16 d,which is consistent with the currently recommended value;however,the uncertainty assessment of the latter was barely documented.In addition,this study indicates that the half-life of the ground state can be obtained by eliminating the contamination of γ-rays emitted from the isomer,which provides the possibility of determining the half-lives of nuclides containing isomers.更多还原

【Abstract】 The isomeric ratio of ^184m,gRe and the half-life of ^184gRe were measured in the ¹⁸⁵Re（n,2n） ¹⁸⁴Re reaction at 14.8 MeV,and the uncertainty was discussed in detail.The measurements were performed using the activation method implemented for a rhenium sample using the K-400 neutron generator at the Chinese Academy of Engineering Physics（CAEP）.Isomeric state and ground state nuclei of ¹⁸⁴Re were identified by their γ-ray spectra.To eliminate the effect of the γ-ray emitted from the isomer on the counting of the ground state characteristic peaks,the isomeric ratio of ^184m,gRe was calculated to be 0.29±0.11 according to the neutron activation cross-section formula.This result is consistent with previous data within the uncertainty and can be used to determine parameters that characterize the dependence of the level density on the excitation energy and angular momentum.Through exponential function fitting and a detailed discussion of the uncertainty evaluation,the half-life of ^184gRe was determined as 35.43 ± 0.16 d,which is consistent with the currently recommended value;however,the uncertainty assessment of the latter was barely documented.In addition,this study indicates that the half-life of the ground state can be obtained by eliminating the contamination of γ-rays emitted from the isomer,which provides the possibility of determining the half-lives of nuclides containing isomers.更多还原