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生物炭的投加对曝气人工湿地中N2O主要产排途径的影响
Influences of biochar on the main production and discharge pathways of N2O in aerated constructed wetlands
【摘要】 生物炭由于具有良好的微孔结构,较大的比表面积,被用于改善人工湿地内部环境,可实现强化脱氮和氧化亚氮(N2O)减排,但生物炭对N2O减排的途径尚不明晰。通过在温室内构建生物炭曝气潜流湿地(BW),以曝气潜流湿地(CK)作为对照,采用化学抑制剂法,量化湿地中N2O的排放途径,探究生物炭对N2O的减排效应。结果表明,生物炭投加可以显著提高湿地脱氮效率(p<0.05)。CK和BW系统N2O的平均释放量分别为17.62 mg·(m2·d)-1和10.45 mg·(m2·d)-1,30%的生物炭投加可实现N2O减排40.69%。化学抑制剂实验表明,湿地系统中硝化和反硝化作用对N2O释放的贡献率分别为43.48%和34.81%。生物炭的添加可使上述2个主要脱氮过程的N2O减排43.20%和71.93%。本研究可为污水处理流程的碳减排提供参考。
【Abstract】 Biochar is used to improve the internal environment of constructed wetlands, achieving nitrogen removal enhancement and nitrous oxide(N2O) emission reduction, due to the microporous structure and huge specific surface area. However, the way of N2O emission reduction by biochar is not clear yet. In this experiment, the aeration subsurface flow constructed wetland with biochar(BW) was built in the greenhouse,using the one without biochar(CK) as control. The chemical inhibitor method was used to quantify the N2O emission pathway and explore the reduction effects of biochar on N2O. The results revealed that biochar addition could significantly improve the nitrogen removal efficiency(p <0.05). The average release of N2O in CK and BW were 17.62 mg·(m2·d)-1 and 10.45 mg·(m2·d)-1, respectively, and 30% biochar addition would reduce N2O emissions by 40.69%. Chemical inhibitor tests showed that the contribution of nitrification and denitrification to N2O release were 43.48% and 34.81%, and the addition of biochar could reduce the N2O emission by 43.20%and 71.93%, respectively, in these two major nitrogen removal processes.
【Key words】 constructed wetland; biochar; nitrogen removal; nitrous oxide; chemical inhibition;
- 【文献出处】 环境工程学报 ,Chinese Journal of Environmental Engineering , 编辑部邮箱 ,2022年11期
- 【分类号】X703
- 【下载频次】17