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苛性碱吸收模拟燃煤电厂烟气CO2性能研究

Absorption Performance of Caustic Solution for CO2 Capture from Simulated Flue Gas in Coal-fired Power Plant

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【作者】 王亮刘飞厉宸希祁志福翁建明杨睿刘羽申震

【Author】 WANG Liang;LIU Fei;LI Chenxi;QI Zhifu;WENG Jianming;YANG Rui;LIU Yu;SHEN Zhen;Zhejiang Zheneng Jiahua Electric Power Generation Co., Ltd.;Zhejiang Energy Group R&D Institute Co., Ltd.;Engineering Research Center for New Industrial Water Resources of Zhejiang Province;State Key Laboratory of Clean Energy Utilization, Zhejiang University;Key Laboratory of Solar Energy Utilization & Energy Saving Technology of Zhejiang Province;

【通讯作者】 申震;

【机构】 浙江浙能嘉华发电有限公司浙江浙能技术研究院有限公司工业新水源技术浙江省工程研究中心浙江大学清洁能源利用国家重点实验室浙江省太阳能利用及节能技术重点实验室

【摘要】 以散堆填料吸收塔作为反应器,采用单因素分析方法研究了吸收液进口温度、吸收当量比、停留时间和吸收液浓度等因素对CO2捕集的影响,并采用正交试验对这些参数进行优化。结果表明:在实验条件下,各因素对CO2捕集影响由大到小依次为吸收液进口温度、停留时间、吸收当量比和吸收液浓度;吸收液进口温度与停留时间对CO2捕集有显著影响,吸收当量比和吸收液浓度对CO2捕集影响较小;最佳工况组合为吸收液进口温度为40℃,停留时间为5 s,吸收当量比为100%,吸收液浓度为2.0 mol/L。

【Abstract】 Effect of absorbent inlet temperature, equivalence ratio, residence time, concentration of NaOH solution on CO2 capture in a random packed absorber reactor was studied by single-factor experiments, and these parameters were optimized using orthogonal test. Results show that under the experimental conditions, the effects on CO2 capture is in a descending sequence as inlet temperature, residence time, equivalence ratio and concentration. Both inlet temperature and residence time of NaOH solution have obvious influence on CO2 capture while minor effect of equivalence ratio and concentration exist. The optimum conditions are achieved at inlet temperature of 40 ℃, residence time of 5 s, equivalence ratio of 100%, and NaOH concentration of 2.0 mol/L.

【基金】 国家自然科学基金资助项目(51776182)
  • 【文献出处】 动力工程学报 ,Journal of Chinese Society of Power Engineering , 编辑部邮箱 ,2022年08期
  • 【分类号】X773
  • 【被引频次】1
  • 【下载频次】109
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