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纳米限域催化剂在高级氧化水处理中的应用研究进展

Research Advances in the Application of Nanoconfined Catalysts in Advanced Oxidation Water Treatment

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【作者】 郭东丽赵志远尤世界刘艳彪

【Author】 GUO Dongli;ZHAO Zhiyuan;YOU Shijie;LIU Yanbiao;Textile Pollution Controlling Engineering Center of Ministry of Environmental Protection, College of Environmental Science and Engineering, Donghua University;State Key Laboratory of Urban Water Resource and Environment, School of Environment, Harbin Institute of Technology;Shanghai Institute of Pollution Control and Ecological Security;

【通讯作者】 刘艳彪;

【机构】 东华大学环境科学与工程学院国家环境保护纺织工业污染防治工程技术中心哈尔滨工业大学环境学院城市水资源与水环境国家重点实验室上海污染控制与生态安全研究院

【摘要】 近年来,纳米限域催化剂由于其独特的结构和理化特性引起了广泛关注,有望通过其解决传统催化氧化水处理过程所面临的催化剂活性低和稳定性差等问题。为进一步深化对纳米限域催化的认识,本文回顾了纳米限域催化剂在不同高级氧化水处理过程中的应用研究进展,归纳了水处理过程中独特的“纳米限域效应”和载体材料的理化特性,总结了纳米限域催化剂在不同高级氧化体系中的催化氧化新机理。最后,提出了纳米限域催化剂在高级氧化水处理过程中面临的挑战及未来发展方向。

【Abstract】 Recently, nanoconfined catalysts have been extensively investigated toward advanced water treatment due to their unique structure and physicochemical attributes, through which the long-lasting challenges may get addressed like low catalytic activity and poor stability in conventional catalytic oxidation systems. To deepen the understanding on nanoconfined catalysts, herein, we systematically reviewed the research advances of nanoconfined catalysts in different advanced water treatment systems, summarized the unique “nanoconfinement effect” in water treatment processes and the desirable characteristics of various host materials, revealed the new catalytic oxidation mechanisms of nanoconfined catalysts in different advanced oxidation systems. Finally, existing challenges and future prospects of nanoconfined catalysis in advanced water treatment were presented.

【基金】 国家自然科学基金(52170068;U21A20161)~~
  • 【分类号】TQ426;TB383.1
  • 【下载频次】289
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