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复合光催化剂TS-1的制备及降解四环素的性能研究

Preparation of TS-1 composite photocatalyst and its performance in degradation of tetracycline

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【作者】 相丹丹郭一帆申文静郭泉辉马新起汤雁婷

【Author】 XIANG Dandan;GUO Yifan;SHEN Wenjing;GUO Quanhui;MA Xinqi;TANG Yanting;College of Chemistry and Chemical Engineering, Henan University;Henan Engineering Research Center of Resource and Energy Recovery from Waste, Henan University;

【通讯作者】 汤雁婷;

【机构】 河南大学化学化工学院河南大学河南省废弃物资源能源化工程技术研究中心

【摘要】 基于水热合成法制备的纯硅分子筛Silicalite-1为载体,采用溶胶凝胶法制备了TiO2-Silicalite-1复合光催化剂,以降解率为对象考察了对四环素的光催化降解性能.用扫描电镜(SEM)、紫外可见漫反射光谱(UV-vis)、X射线衍射(XRD)、X射线荧光光谱仪(XRF)等对复合光催化剂进行了表征.以四环素为模拟污染物,选择了在300 W氙灯的照射下,催化剂用量为0.5 mg/L时,探讨了TiO2-Silicalite-1光催化降解四环素的性能.实验结果表明,最优组合催化剂对四环素的降解率达87.3%.

【Abstract】 The pure silicon zeolite Silicalite-1 was synthesized by hydrothermal synthesis, and then the TiO2-Silicalite-1 composite photocatalyst was prepared by sol-gel method using Silicalite-1 as carrier. The degradation rate of tetracycline was investigated by photocatalytic degradation. The composite photocatalyst was characterized by SEM, UV-Vis, XRD and XRF. The photocatalytic degradation of tetracycline by TiO2-silicalite-1 was studied when the amount of catalyst was 0.5 mg/L under the irradiation of 300 W xenon lamp. The results showed that the degradation rate of tetracycline was 87.3%.

【基金】 河南省科技发展计划项目(202102310606)
  • 【分类号】X703;TQ426
  • 【下载频次】152
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