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石墨相氮化碳基Z-Scheme体系光催化分解水研究进展

Progress on g-C3N4-based Z-Scheme photocatalytic system for photocatalytic water splitting

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【作者】 时晓羽李会鹏赵华张杰

【Author】 Shi Xiaoyu;Li Huipeng;Zhao Hua;Zhang Jie;Division of Chemistry,Chemical Engineering and Environment,Liaoning Shihua University;

【通讯作者】 李会鹏;

【机构】 辽宁石油化工大学化学化工与环境学部

【摘要】 石墨相氮化碳(g-C3N4)以独特的电子结构、稳定的化学结构和显著的可见光活性而备受瞩目,g-C3N4基Z-Scheme光催化体系能够有效地降低光生电子空穴的复合几率,提高光源吸收利用率。介绍了光催化分解水的反应机理,综述了g-C3N4基Z-Scheme体系在光催化水氧化、光催化水解制氢、光催化全分解水方面的应用,并对未来Z-Scheme的发展进行了展望。

【Abstract】 Graphitic carbon nitride(g-C3N4),with unique electronic structure,high stability,and visible-light-induced photocatalytic activity,has attracted considerable attention. The g-C3N4-based Z-scheme photocatalytic system can effectively lower the recombination rate of electron-holes and the utilization of light sources is improved. The reaction mechanism of photocatalytic water splitting and the applications of g-C3N4-based Z-scheme photocatalytic system in photocatalytic water oxidation,photocatalytic water conversion and photocatalytic overall water splitting are reviewed. Moreover,the future development of Z-scheme is forecasted.

  • 【文献出处】 石油化工 ,Petrochemical Technology , 编辑部邮箱 ,2019年09期
  • 【分类号】O643.36;O644.1;TQ116.2
  • 【被引频次】4
  • 【下载频次】296
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