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Bi2WO6复合g-C3N4的制备及其光催化降解甲苯的研究

Preparation of Bi2WO6 Composite g-C3N4 and Study on Its Photocatalytic Degradation of Toluene

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【作者】 王琪曾曦刘心中

【Author】 WANG Qi;ZENG Xi;LIU Xin-zhong;College of Ecological Environment and Urban Construction, Fujian University of Technology;College of Environment and Resources, Fuzhou University;

【通讯作者】 刘心中;

【机构】 福建工程学院生态环境与城市建设学院福州大学环境与资源学院

【摘要】 通过高温热解三聚氰胺制备石墨相氮化碳,再利用水热法合成不同Bi2WO6含量的Bi2WO6-CN复合材料体系并进行了光催化降解实验,利用一系列表征方法对其结构表征。对Bi2WO6的复合量、催化剂投放量以及光照强度等对光催化性能的影响因素进行了考察。结果表明,Bi2WO6与g-C3N4成功复合到了一起,形成异质结,且明显提高了光催化性能。在Bi2WO6的复合量、催化剂投放量以及光照强度分别为60%、100mg和光距15cm的条件下,制备的改性石墨相氮化碳对甲苯的光催化降解率可达72%。

【Abstract】 The graphite phase carbon nitride is prepared by pyrolysis of melamine at high temperature, and the Bi2WO6-CN composite systems with different Bi2WO6 contents are synthesized by hydrothermal method. A series of characterization methods are used to characterize the structure.The influencing factors on the photocatalytic performance are researched, such as the composite amount of Bi2WO6, the amount of catalyst and the light intensity. The results show that the Bi2WO6 and g-C3N4 are successfully combined to form a heterojunction, and the photocatalytic performance has obviously improved. When the composite amount of Bi2WO6, catalyst dosage and light distance is 60%, 100 mg and 15 cm respectively, the modified graphite phase carbon nitride’s photocatalytic degradation rate of toluene can reach 72%.

【关键词】 Bi2WO6g-C3N4光催化甲苯
【Key words】 Bi2WO6g-C3N4photocatalytictoluene
【基金】 福建省科技厅计划资助项目(编号:2016H6002);福建工程学院科研启动基金资助项目(编号:GY-214016,GYZ16007)
  • 【文献出处】 化学与粘合 ,Chemistry and Adhesion , 编辑部邮箱 ,2019年05期
  • 【分类号】TQ426;X701
  • 【被引频次】5
  • 【下载频次】504
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