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Sr-TiO2/多孔陶瓷滤球复合光催化剂对难降解有机物腐殖酸的去除性能

Removal of refractory organic compound humic acid by Sr-TiO2/PCFM photocatalyst

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【作者】 韩帆张义Trinh Xuantung刘子森徐栋贺锋吴振斌

【Author】 Han Fan;Zhang Yi;Trinh Xuantung;Liu Zisen;Xu Dong;He Feng;Wu Zhenbin;School of Resource & Environmental Engineering,Wuhan University of Technology;State Key Laboratory of Freshwater Ecology and Biotechnology,Institute of Hydrobiology,Chinese Academy of Sciences;University of Chinese Academy of Sciences;

【通讯作者】 张义;

【机构】 武汉理工大学资源与环境工程学院中国科学院水生生物研究所淡水生态和生物技术国家重点实验室中国科学院大学

【摘要】 腐殖酸(HA)是自然环境中广泛存在的大分子难降解有机物。以多孔陶瓷滤球(PCFM)为载体,通过溶胶-凝胶法掺杂稀土元素Sr制备出复合光催化剂Sr-TiO2/PCFM,用以降解腐殖酸废水。结果表明:当HA初始浓度为20mg/L,pH=5.98,温度为37℃时,Sr-TiO2/PCFM对HA的降解率可达到86.82%。Sr-TiO2/PCFM重复利用3次后,对HA的降解率仍可维持在40%以上。

【Abstract】 Humic acid(HA)is a kind of refractory organics which widely existed in natural environment.The nano-TiO2 film coated on porous ceramic filter media(PCFM)was prepared by sol-gel process and formed Sr-TiO2/PCFM multiplex photocatalyst,the degrade effect of HA with the photocatalyst was studied.The results showed that the degradation rate of HA could reach 86.82% when the initial concentration of HA was 20 mg/L,pH 5.98 and temperature 37℃.The degradation rate of HA was still more than 40% after Sr-TiO2/PCFM reused for three times.

【关键词】 腐殖酸TiO2多孔陶瓷滤球
【Key words】 humic acidTiO2porous ceramic filter media
【基金】 国家自然科学基金(51709254)
  • 【文献出处】 化工新型材料 ,New Chemical Materials , 编辑部邮箱 ,2019年03期
  • 【分类号】O643.36;O644.1;X703
  • 【被引频次】2
  • 【下载频次】288
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