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具有水下超疏油性能的MXene高效油水分离膜
MXene-Coated Mesh Membrane with Underwater Superoleophobicity for High-efficiency Oi-| water Separation
【摘要】 基于二维材料MXene(Ti3C2Tx)的化学组成和纳米片状结构,在不锈钢网上制备了具有MXene微纳结构表面的新型亲水和水下超疏油分离膜.对于不同类型的油-水混合物,该膜材料可实现重力驱动的高效油水分离,收集的水中残油量小于4 mg/L,具有高分离效率(>99. 99%),水通量高达57. 52 L·m-2·s-1.此外,经高温处理和多种有机溶剂浸泡后MXene膜仍具有高效的油水分离性能,并表现出优异的稳定性和循环性.
【Abstract】 Owing to the hydrophilicity and flake-like structure of the two-dimensional( 2D) MXene( Ti3C2Tx),the 2D MXene nanosheets were coated onto the stainless steel mesh to fabricate a novel hydrophilic and underwater superoleophobic mesh membrane with a corrugated micro-and nanostructure surface. For a series of oil-water mixtures,the MXene-caoted mesh membrane can achieve gravity-driven highefficiency oil-water separation with excellent separation efficiency of over 99.99%,residual oil content of less than 4 mg/L in collected water,and water flux up to 57. 52 L·m-2·s-1. In addition,MXene-coated mesh membranes display outstanding stability and cycleability.
【Key words】 2D nanosheet; MXene-coated mesh membrane; Underwater superoleophobicity; Oil-water separation;
- 【文献出处】 高等学校化学学报 ,Chemical Journal of Chinese Universities , 编辑部邮箱 ,2019年04期
- 【分类号】TQ051.893
- 【被引频次】9
- 【下载频次】880