节点文献
高剪切反应器中有机相强化KHCO3/K2CO3溶液吸收CO2研究
Study on CO2 absorption into KHCO3/K2CO3 solution intensified by organic phase in a high shear reactor
【摘要】 在高剪切反应器(HSR)中研究了不同有机分散相对KHCO3/K2CO3溶液吸收CO2的强化效果,并考察了有机相与有机胺溶液复配使用对CO2吸收率的影响。实验结果表明:环己烷、正庚烷对KHCO3/K2CO3溶液吸收CO2的强化效果明显,甲苯、正辛醇对KHCO3/K2CO3溶液吸收CO2则没有明显的强化效果;CO2吸收率随HSR转速的增加而增加,随气液比、温度的增加而降低;环己烷对加入二乙醇胺活化的K2CO3溶液有较为明显的强化作用,CO2吸收率最高可提高23%。与文献中不同反应器的对比表明HSR对CO2具有较高的吸收效率。
【Abstract】 The intensification effect of different organic phases on the absorption of CO2 by KHCO3/K2CO3 solution in a high shear reactor(HSR) was investigated, and the combined effect of organic phase with organic amine on CO2 absorption was also studied. The experimental results showed that cyclohexane and n-heptane exhibited significant intensification effect on the absorption of CO2 by KHCO3/K2CO3 solution, while the intensification effect of toluene and n-octanol on CO2 absorption by KHCO3/K2CO3 solution was negligible. CO2 absorption percentage increased with the increase in the rotation speed of HSR and decreased with increasing gas-liquid ratio and temperature. CO2 absorption by diethanolamine-activated K2CO3 solution was significantly enhanced by the addition of cyclohexane, with an increase of CO2 absorption percentage up to 23%. HSR demonstrated a high efficiency for CO2 absorption by a comparison with other reactors in the literature.
【Key words】 gas-liquid-liquid system; CO2 absorption; high shear reactor; enhancement factor;
- 【文献出处】 北京化工大学学报(自然科学版) ,Journal of Beijing University of Chemical Technology(Natural Science Edition) , 编辑部邮箱 ,2019年01期
- 【分类号】TQ028.14
- 【被引频次】4
- 【下载频次】98