节点文献

耦合原料气预热的Sabatier固定床反应器拉偏试验研究

Experimental Condition Study of Sabatier Fixed-bed Reactor Coupled with Feed Gas Preheating

  • 推荐 CAJ下载
  • PDF下载
  • 不支持迅雷等下载工具,请取消加速工具后下载。

【作者】 段洪敏侯宝林吉定豪苏雄黄延强张涛

【Author】 DUAN Hongmin;HOU Baolin;JI Dinghao;SU Xiong;HUANG Yanqiang;ZHANG Tao;Dalian Institute of Chemical Physics,Chinese Academy of Sciences;China Astronaut Research and Training Center;

【机构】 中国科学院大连化学物理研究所中国航天员科研训练中心

【摘要】 CO2还原是长期载人航天中生命保障系统的关键技术,针对作为CO2还原系统核心的反应器及其中的催化剂的效率问题,在耦合原料气预热的Sabatier固定床反应器和Ru/Al2O3催化剂上,在宽范围的原料气氢碳比(1∶15∶1)和流量(28 L/min)工况下,进行了Sabatier反应拉偏试验,结果表明:反应的起动温度为150℃,在不同原料气流量和氢碳比下,反应器温度梯度分布合理,贫组分的转化率达到98%以上(氢碳比4∶1除外)。耦合原料气预热的Sabatier固定床反应器结构合理,Ru/Al2O3催化剂活性高,能够高效处理舱室中24人的代谢量。

【Abstract】 The CO2 reduction is one of the key technologies of the life-support system in long duration manned space flight. The reactor is the hard core of the CO2 reduction system. Sabatier reaction was tested under the H2/CO2 ratio from 1 ∶ 1 to 5 ∶ 1 and the flow rate of feed gas between 2. 0 8. 0 L/min in a Sabatier fixed-bed reactor coupled with feed gas preheating filled with Ru/Al2O3 catalysts. The reaction was started successfully at 150 ℃,and the distribution of temperature steps in the reactor was regular under different conditions. The conversion of the lean component reached above 98% except for the ratio of H2 to CO2( 4∶ 1). The configuration of the Sabatier fixed-bed reactor coupled with feed gas preheating was reasonable,and the activity of Ru/Al2O3 catalysts was high. The favorable performance was achieved for a crew size of 2 4 persons in the cabin.

【基金】 国家自然科学基金(21676266)
  • 【文献出处】 载人航天 ,Manned Spaceflight , 编辑部邮箱 ,2017年01期
  • 【分类号】V444.3
  • 【被引频次】2
  • 【下载频次】104
节点文献中: 

本文链接的文献网络图示:

本文的引文网络