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大气气溶胶中的氮:化学形态与同位素特征研究进展

Research progress on nitrogen in atmospheric aerosols:Chemical speciation and isotopic characteristics

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【作者】 李佩霖傅平青康世昌万欣刘彬邬光剑丛志远

【Author】 LI Peilin;FU Pingqing;KANG Shichang;WAN Xin;LIU Bin;WU Guangjian;CONG Zhiyuan;Key Laboratory of Tibetan Environment Changes and Land Surface Processes,Institute of Tibetan Plateau Research,Chinese Academy of Sciences;University of Chinese Academy of Sciences;State Key Laboratory of Atmospheric Boundary Layer Physics and Atmospheric Chemistry,Institute of Atmospheric Physics,Chinese Academy of Sciences;State Key Laboratory of Cryospheric Sciences,Cold and Arid Regions Environmental and Engineering Research Institute,Chinese Academy of Sciences;

【机构】 中国科学院青藏高原研究所青藏高原环境变化与地表过程重点实验室中国科学院大学中国科学院大气物理研究所大气边界层物理和大气化学国家重点实验室中国科学院寒区旱区环境与工程研究所冰冻圈科学国家重点实验室

【摘要】 氮是大气气溶胶的重要组成部分.气溶胶中的氮组分参与大气中的光化学反应,进而改变大气组成,影响气候变化与人类健康.同时,大气中过量的颗粒氮改变了氮素的自然循环,当它们沉降到地表时对陆地和水生生态系统产生深远的影响.本文综述了近年来气溶胶氮组分的研究进展,按其化学形态分别阐述了气溶胶中无机氮和有机氮的来源及其相关大气化学过程等,同时探讨了气溶胶中氮的同位素特征,指出该研究领域的薄弱环节并对其研究前景进行了展望.

【Abstract】 As a key component,nitrogen constituents in atmospheric aerosols can participate in the atmospheric photochemical reactions and thereby altering the atmospheric composition. They can also exert great influence on the climate and human health. Excessive levels of atmospheric particulate nitrogen have profoundly changed the natural nitrogen cycle. Furthermore,after the deposition,it has dramatically affected the terrestrial / aquatic ecosystems. In this review,the research progress on nitrogen in atmospheric aerosols is summarized in terms of the chemical composition of inorganic /organic nitrogen,their sources and related atmospheric chemical processes,and the nitrogen isotopic compositions. Lastly,the shortcomings of previous researches and the future research prospective are discussed.

【基金】 国家自然科学基金(41271073;41225002;41501082);中国科学院战略性先导科技专项:应对气候变化的碳收支认证及相关问题(XDA05100105)资助~~
  • 【文献出处】 环境化学 ,Environmental Chemistry , 编辑部邮箱 ,2016年01期
  • 【分类号】X513
  • 【被引频次】17
  • 【下载频次】807
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