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Effect of Water Vapor on Toluene Removal in Catalysis-DBD Plasma Reactors

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【作者】 王婧婷曹栩张仁熙龚挺侯惠奇陈善平张瑞娜

【Author】 WANG Jingting;CAO Xu;ZHANG Renxi;GONG Ting;HOU Huiqi;CHEN Shanping;ZHANG Ruina;Shanghai Key Laboratory of Atmospheric Particle Pollution and Prevention(LAP3),Department of Environmental Science & Engineering,Fudan University;Shanghai Institute for Design & Research on Environmental Engineering;

【机构】 Shanghai Key Laboratory of Atmospheric Particle Pollution and Prevention(LAP3),Department of Environmental Science & Engineering,Fudan UniversityShanghai Institute for Design & Research on Environmental Engineering

【摘要】 The experiment was carried out in a cylindrical dielectric barrier discharge(DBD)reactor assisted with a catalyst to decompose toluene under different humidity.In order to explore the synergistic effect on removing toluene in the catalysis-DBD reactor,this paper investigated the decomposition efficiency and the energy consumption in the catalysis-DBD and the non-catalyst DBD reactors under different humidity.The results showed that the catalysis-DBD reactor had a better performance than the non-catalysis one at the humidity ratio of 0.4%,and the removal efficiency of toluene could reach 88.6% in the catalysis-DBD reactor,while it was only 59.9% in the non-catalytic reactor.However,there was no significant difference in the removal efficiency of toluene between the two reactors when the humidities were 1.2% and 2.4%.Additionally,the degradation products were also analyzed in order to gain a better understanding of the mechanism of decomposing toluene in a catalysis-DBD reactor.

【Abstract】 The experiment was carried out in a cylindrical dielectric barrier discharge(DBD)reactor assisted with a catalyst to decompose toluene under different humidity.In order to explore the synergistic effect on removing toluene in the catalysis-DBD reactor,this paper investigated the decomposition efficiency and the energy consumption in the catalysis-DBD and the non-catalyst DBD reactors under different humidity.The results showed that the catalysis-DBD reactor had a better performance than the non-catalysis one at the humidity ratio of 0.4%,and the removal efficiency of toluene could reach 88.6% in the catalysis-DBD reactor,while it was only 59.9% in the non-catalytic reactor.However,there was no significant difference in the removal efficiency of toluene between the two reactors when the humidities were 1.2% and 2.4%.Additionally,the degradation products were also analyzed in order to gain a better understanding of the mechanism of decomposing toluene in a catalysis-DBD reactor.

【基金】 supported by the Key Project which is sponsored by the Science and Technology Commission of Shanghai Municipality(No.13231201903);the Key Programs for Science and Technology Development sponsored by the Science and Technology Commission of Shanghai Municipality(Nos.13231201901 and 14DZ1208401);the Key Project sponsored by the State-owned Assets Supervision and Administration Commission of Shanghai,China(No.2013019)
  • 【文献出处】 Plasma Science and Technology ,等离子体科学和技术(英文版) , 编辑部邮箱 ,2016年04期
  • 【分类号】X701;TQ052
  • 【被引频次】7
  • 【下载频次】74
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