Photon Statistical Properties of Single Terrylene Molecules in P-Terphenyl Crystals

【摘要】 We consider the photon emission statistical properties of a single molecule under pump-probe field driving,using the generating function method.The first- and second-order moments of statistical quantities are presented.Derived from the first-order moment,the line shapes are in good agreement with the experimental results.Derived from the second-order moment,Mandel’s Q parameters show an obvious quantum effect of photon statistical distribution,i.e.,the anti-bunching effect.更多还原

【Abstract】 We consider the photon emission statistical properties of a single molecule under pump-probe field driving,using the generating function method.The first- and second-order moments of statistical quantities are presented.Derived from the first-order moment,the line shapes are in good agreement with the experimental results.Derived from the second-order moment,Mandel’s Q parameters show an obvious quantum effect of photon statistical distribution,i.e.,the anti-bunching effect.更多还原