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液闪三双符合比方法测量99Tc放射性活度

Standardization of 99Tc by the Triple-to-double Coincidence Ratio( TDCR) Method of Liquid Scintillation Counting

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【作者】 吴永乐刘浩然柳加成李宏宇梁珺成熊文俊姚顺和陈细林杨元第袁大庆

【Author】 WU Yong-le;Liu Hao-ran;LIU Jia-cheng;Li Hong-yu;LIANG Jun-cheng;XIONG Wen-jun;YAO Shun-he;CHEN Xi-lin;YANG Yuan-di;YUAN Da-qing;China Institute of Atomic Energy;Nuclear and Radiation Safety Center;National Institute of Metrology;

【机构】 环保部核与辐射安全中心中国原子能科学研究院中国计量科学研究院

【摘要】 液闪三双符合比(TDCR)方法采用3个光电倍增管对称放置的液闪计数器,利用三管符合和三对两管符合的计数计算液闪探测效率,从而得到放射性活度,不需要使用标准源对仪器进行效率刻度,是一种放射性活度绝对测量方法。由于具有无自吸收、制源简单、操作简便、一致性好等优点,已广泛应用于纯β衰变核素放射性活度的测量。介绍了液闪TDCR方法的基本原理和液闪TDCR活度测量装置,并绝对测量了纯β衰变核素99Tc放射性活度,测量不确定度小于0.3%。

【Abstract】 The triple- to- double coincidence ratio( TDCR) method is a kind of primary measurement method of radioactivity,requiring the use of a liquid scintillation counter equipped with of 3 photomultiplier tubes. The counting efficiency calculated through the triple coincidence count and 3 double coincidence counts. Due to its advantages in simple sample preparation,no self- absorption and good consistency,the TDCR method is a popular technique for the standardization of pure beta radionuclides. The principle of TDCR method is described in this paper. And a sample of99 Tc is calibrated in term of specify activity on the newly established TDCR system with uncertainty within 0. 3%.

  • 【文献出处】 核电子学与探测技术 ,Nuclear Electronics & Detection Technology , 编辑部邮箱 ,2014年04期
  • 【分类号】TL812.2
  • 【被引频次】2
  • 【下载频次】169
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