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Evaluation of metal-doped manganese oxide octahedral molecular sieves in catalytic reduction of NO_x from cigarette mainstream smoke

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【作者】 练文柳任凤莲刘琦谢兰英

【Author】 LIAN Wen-liu1,2,REN Feng-lian1,LIU Qi2,XIE Lan-ying2 1.School of Chemistry and Chemical Engineering,Central South University,Changsha 410083,China;2.Research Center of China Tobacco Hunan Industrial Co.,Ltd.,Changsha 410014,China

【机构】 School of Chemistry and Chemical Engineering,Central South UniversityResearch Center of China Tobacco Hunan Industrial Co.,Ltd.

【摘要】 A series of Ag,Cu and Co-doped manganese oxide octahedral molecular sieves(OMS-2) were synthesized and evaluated to remove nitrogen oxides(NOx) from cigarette mainstream smoke.The three kinds of catalysts were added to cigarettes for studying the capabilities of reducing NOx from cigarette mainstream smoke.The catalysis and reduction of NO in laboratory were studied.A mechanism for NOx catalytic reduction from burning cigarettes with the catalysts adding to cigarettes was described.The catalysts show excellent catalytic activity for NOx removal,especially the Ag-doped OMS-2 catalyst.0.5%(mass fraction) Ag-doped OMS-2 catalyst has the best ability to remove NOx from cigarette mainstream smoke.The use of Ag-doped OMS-2 as catalyst for removing carcinogenic compounds from cigarette smoke will be an effective strategy to protect the environment and public health.

【Abstract】 A series of Ag,Cu and Co-doped manganese oxide octahedral molecular sieves(OMS-2) were synthesized and evaluated to remove nitrogen oxides(NOx) from cigarette mainstream smoke.The three kinds of catalysts were added to cigarettes for studying the capabilities of reducing NOx from cigarette mainstream smoke.The catalysis and reduction of NO in laboratory were studied.A mechanism for NOx catalytic reduction from burning cigarettes with the catalysts adding to cigarettes was described.The catalysts show excellent catalytic activity for NOx removal,especially the Ag-doped OMS-2 catalyst.0.5%(mass fraction) Ag-doped OMS-2 catalyst has the best ability to remove NOx from cigarette mainstream smoke.The use of Ag-doped OMS-2 as catalyst for removing carcinogenic compounds from cigarette smoke will be an effective strategy to protect the environment and public health.

  • 【文献出处】 Journal of Central South University ,中南大学学报(英文版) , 编辑部邮箱 ,2012年04期
  • 【分类号】X511
  • 【被引频次】3
  • 【下载频次】42
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