节点文献

环丁砜-二乙醇胺(DEA)复合溶液吸收烟气中CO2

Experiment research of Sulfolane-DEA mixed amine solutions absorbing carbon dioxide from flue gas

  • 推荐 CAJ下载
  • PDF下载
  • 不支持迅雷等下载工具,请取消加速工具后下载。

【作者】 张艳李清方陆诗建曲虎刘英超闫丹丹

【Author】 ZHANG Yan1,2,LI Qing-fang1,LU Shi-jian1,QU Hu2,LIU Ying-chao2,YAN Dan-dan2(1.Shengli Engineering & Consulting co.ltd.,Dongying 257026,China;2.College of Chemistry & Chemical Engineering in China University of Petroleum,Dongying 257061,China)

【机构】 胜利油田勘察设计研究院中国石油大学〈华东〉

【摘要】 采用搅拌实验装置,研究不同配比的环丁砜-DEA复合溶液对烟道气中二氧化碳的吸收和解吸性能,揭示了吸收速率、吸收容量与酸碱度、时间之间的内在联系,并对CO2初始逸出温度、试液再生温度、试液再生率、再生pH下降率进行了细致记录分析.实验结果表明:环丁砜-DEA复合溶液配比为0.1 0.9时:吸收效果最佳,吸收量约为0.253 mol;再生温度最低,约为102.2℃,再生率为87.17%.实验结果也说明该复合体系之间存在负的交互作用.

【Abstract】 A set of Stirring experiment was used to study the capability of absorption and desorption of carbon dioxide from flue gas with Sulfolane-DEA complex solution.The study revealed the releationship between absorption rate,absorption capacity,pH and time.Meanwhile,the data was recorded and analyzed,including the initial escape temperature of CO2,regeneration temperature,regeneration rate,and pH decline rate in regeneration.Experimental results showed that the absorption effect was the best in which the absorption capacity was 0.253 mol,when binary complex system SulfolaneDEA was 0.60.4.The highest regeneration rate was about 87.17% at the lowest regeneration temperature 106 ℃.The results also showed the negative interaction between potassium carbonate and TETA solution existed.

【关键词】 二氧化碳环丁砜-二乙醇胺吸收解吸
【Key words】 carbon dioxidesulfolane-DEAabsorptiondesorption
【基金】 国家科技支撑计划项目(NO.2008BAE65B00)
  • 【文献出处】 武汉工程大学学报 ,Journal of Wuhan Institute of Technology , 编辑部邮箱 ,2011年08期
  • 【分类号】X701
  • 【被引频次】4
  • 【下载频次】189
节点文献中: 

本文链接的文献网络图示:

本文的引文网络