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磁制冷材料Gd5Ge4中的磁玻璃态(英文)

The magnetic glass state in the magnetocaloric material Gd5Ge4

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【作者】 董彤袁淑娟葛军饴洪芳郁黎明曹世勋张金仓

【Author】 DONG Tong1,YUAN Shu-juan1,2*,GE Jun-yi1,HONG Fang1,YU Li-ming1,CAO Shi-xun1,ZHANG Jin-cang1(1.Department of Physics,Shanghai University,Shanghai 200444,China;2.Laboratory of Solid State Microstructures,Nanjing University,Nanjing 210093,China)

【机构】 上海大学物理系南京大学固体微结构实验室

【摘要】 Gd5Ge4低温时具有玻璃态的不稳定性,与钴氧化物La0.88Sr0.12CoO3的冻结的自旋玻璃态不同.通过分别研究经过零场冷过程后Gd5Ge4和La0.88Sr0.12CoO3在低温区域的温度循环对磁化强度的影响,发现在Gd5Ge4样品中磁化强度随着温度循环的增加而不断增大,但是在La0.88Sr0.12CoO3样品中温度循环对其磁化强度几乎没有影响.Gd5Ge4和La0.88Sr0.12CoO3的直流磁化强度和交流磁化率也进行了测量.Gd5Ge4的交流磁化率的峰并不随着频率的增加而向高温区移动,这个现象不同于La0.88Sr0.12CoO3样品的.通过不同物理参数的测量,证明了Gd5Ge4的这种磁玻璃态不同于传统的自旋玻璃态.

【Abstract】 The metastable property of glasslike dynamics at low temperature of Gd5Ge4 was presented in contrast to the stable frozen spin glass state in cobaltite La0.88Sr0.12CoO3(LSCO).Through investigating the effect of temperature cycle on magnetization at the low temperature region after the zero field cooled procedure of Gd5Ge4 and La0.88Sr0.12CoO3 respectively,it was found that the magnetization continues to increase with increasing the temperature cycle in Gd5Ge4,while there was hardly any effect on magnetization in La0.88Sr0.12CoO3.The dc magnetization and ac susceptibility were also measured on Gd5Ge4 and La0.88Sr0.12CoO3.The peaks of ac susceptibility in Gd5Ge4 did not move to the higher temperature region with increasing frequency,which were different from the phenomena of La0.88Sr0.12CoO3.This kind of magnetic glass state in Gd5Ge4 is quite different from conventional spin glass.

【基金】 National Natural Science Foundationof China(10504019,10674092);Shanghai Nano-technology Promotion Center and the Science & Technology Committee of Shanghai Municipality(0652nm046).
  • 【文献出处】 山东大学学报(工学版) ,Journal of Shandong University(Engineering Science) , 编辑部邮箱 ,2009年03期
  • 【分类号】TB64
  • 【下载频次】102
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