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Removal of nitrate from groundwater by heterotrophic denitrification using the solid carbon source

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【Author】 WANG XuMing1,2 & WANG JianLong1 1 Laboratory of Environmental Technology,INET,Tsinghua University,Beijing 100084,China;2 College of Plant Science,Jilin University,Changchun 130062,China

【摘要】 Removal of nitrate from groundwater was investigated using biodegradable meal box(BMB) and poly(ε-caprolactone)(PCL) as carbon source and biofilm carrier.The experimental results show that nitrate in groundwater can be effectively removed using BMB and PCL as carbon source.Denitrification rates supported by BMB and PCL were 52.80 and 42.77 mg(NO3-N)/(m2h),respectively,at 30 ℃ and pH 7.5.The pH value of effluent ranged from 7 to 8,and NO2-N concentration was less than 0.1 mg/L.Compared with BMB,PCL could decrease nitrite accumulation;however,more significant influence of temperature on denitrification was observed for PCL as carbon source.Temperature constants for BMB and PCL were 0.045 and 0.068,respectively,at 10-30℃.Based on denitrification efficiency and cost,BMB is more suitable as a carbon source for denitrification of groundwater than PCL.

【Abstract】 Removal of nitrate from groundwater was investigated using biodegradable meal box(BMB) and poly(ε-caprolactone)(PCL) as carbon source and biofilm carrier.The experimental results show that nitrate in groundwater can be effectively removed using BMB and PCL as carbon source.Denitrification rates supported by BMB and PCL were 52.80 and 42.77 mg(NO3-N)/(m2h),respectively,at 30 ℃ and pH 7.5.The pH value of effluent ranged from 7 to 8,and NO2-N concentration was less than 0.1 mg/L.Compared with BMB,PCL could decrease nitrite accumulation;however,more significant influence of temperature on denitrification was observed for PCL as carbon source.Temperature constants for BMB and PCL were 0.045 and 0.068,respectively,at 10-30℃.Based on denitrification efficiency and cost,BMB is more suitable as a carbon source for denitrification of groundwater than PCL.

【基金】 Supported by the National Natural Science Foundation of China (Grant Nos. 59978020 and 50508018);the Specialized Research Fund for the Doctoral Program of Higher Education (Grant No. 20050003023);China Postdoctoral Science Foundation (Grant No. 20070420357)
  • 【文献出处】 Science in China(Series B:Chemistry) ,中国科学(B辑:化学)(英文版) , 编辑部邮箱 ,2009年02期
  • 【分类号】X703
  • 【被引频次】23
  • 【下载频次】94
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