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Catalytic Decomposition of Toluene Using Various Dielectric Barrier Discharge Reactors

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【作者】 叶代启黄海保陈韦丽曾荣辉

【Author】 YE Daiqi HUANG Haibao CHEN Weili ZENG Ronghui College of Environmental Science and Engineering,South China University of Technology,Guangzhou 510640,China

【机构】 College of Environmental Science and Engineering, South China University of Technology, Guangzhou 510640, China

【摘要】 <正> Decomposition of toluene was experimentally investigated with various dielectricbarrier discharge (DBD) reactors,such as wire-cylinder,wire-plate and plate-to-plate,combinedwith multi-metal oxides catalyst (Mn-Ni-Co-Cu-Ox/Al2O3) loaded on the cordierite honeycomband nickel foam,respectively.The effects of some factors including the residence time,reactorconfiguration and catalyst,upon the toluene destruction were studied.Results revealed thatthe use of in-plasma catalysis was more helpful to enhancing the DRE (destruction and removalefficiency) and reducing the O3 formation than that of either post-plasma catalysis or plasmaalone.It was demonstrated that the wire-plate reactor was favorable for the oxidation reaction oftoluene and the nickel foam-supported catalysts exhibited good activity.

【Abstract】 Decomposition of toluene was experimentally investigated with various dielectric barrier discharge (DBD) reactors,such as wire-cylinder,wire-plate and plate-to-plate,combined with multi-metal oxides catalyst (Mn-Ni-Co-Cu-Ox/Al2O3) loaded on the cordierite honeycomb and nickel foam,respectively.The effects of some factors including the residence time,reactor configuration and catalyst,upon the toluene destruction were studied.Results revealed that the use of in-plasma catalysis was more helpful to enhancing the DRE (destruction and removal efficiency) and reducing the O3 formation than that of either post-plasma catalysis or plasma alone.It was demonstrated that the wire-plate reactor was favorable for the oxidation reaction of toluene and the nickel foam-supported catalysts exhibited good activity.

【基金】 National Natural Science Foundation of China(No.20577011);Guangdong Provincial Key Scientific and Technological Project(No.2001367,2002254);Guangzhou Municipal Key Scientific and Technological Project(No.2001-Z-016-01)
  • 【文献出处】 Plasma Science and Technology ,等离子体科学和技术(英文版) , 编辑部邮箱 ,2008年01期
  • 【分类号】O539
  • 【被引频次】9
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